The Influence of Water on the Optical Properties of Single-Layer Molybdenum Disulfide


Varghese JO1, Agbo P1, Sutherland AM1, Brar VW2, George R. Rossman3, Gray HB1, Heath JR1

1Division of Chemistry and Chemical Engineering, California Institute of Technology, Pasadena, CA 91125
2Division of Applied Physics and Materials Science, California Institute of Technology, Pasadena, CA 91125
3Division of Geological and Planetary Sciences, California Institute of Technology, Pasadena, CA 91125


Abstract

Single-layer molybdenum disulfide (SL-MoS2) is a noncentrosymmetric semiconductor with a direct bandgap of about 1.8eV.  Many properties of SL-MoS2 are poorly understood. Weakly bound adsorbates such a physisorbed water may strongly alter its physical properties. Here we quantitatively explore how adsorbed water influences the electrical and photonic properties of SL-MoS2.



Revised 27-Jun-2015